Uncertainty in aerosol-cloud radiative forcing is driven by clean conditions
(2022)
Is anthropogenic global warming accelerating?
Journal of Climate American Meteorological Society 35:24 (2022) 4273-4290
Abstract:
Estimates of the anthropogenic effective radiative forcing (ERF) trend have increased by 50% since 2000 (+0.4W/m2/decade in 2000-2009 to +0.6W/m2/decade in 2010-2019), the majority of which is driven by changes in the aerosol ERF trend, due to aerosol emissions reductions. Here we study the extent to which observations of the climate system agree with these ERF assumptions. We use a large ERF ensemble from IPCC’s Sixth Assessment Report (AR6) to attribute the anthropogenic contributions to global mean surface temperature (GMST), top-of-atmosphere radiative flux, and aerosol optical depth observations. The GMST trend has increased from +0.18°C/decade in 2000-2009 to +0.35°C/decade in 2010-2019, coinciding with the anthropogenic warming trend rising from +0.19°C/decade in 2000-2009 to +0.24°C/decade in 2010-2019. This, and observed trends in top-of-atmosphere radiative fluxes and aerosol optical depths support the claim of an aerosol-induced temporary acceleration in the rate of warming. However, all three observation datasets additionally suggest smaller aerosol ERF trend changes are compatible with observations since 2000, since radiative flux and GMST trends are significantly influenced by internal variability over this period. A zero-trend-change aerosol ERF scenario results in a much smaller anthropogenic warming acceleration since 2000, but is poorly represented in AR6’s ERF ensemble. Short-term ERF trends are difficult to verify using observations, so caution is required in predictions or policy judgments that depend on them, such as estimates of current anthropogenic warming trend, and the time remaining to, or the outstanding carbon budget consistent with, 1.5°C warming. Further systematic research focused on quantifying trends and early identification of acceleration or deceleration is required.Quantifying the impact of meteorological uncertainty on emission estimates and the risk to aviation using source inversion for the Raikoke 2019 eruption
Atmospheric Chemistry and Physics European Geosciences Union 22:13 (2022) 8529-8545
Abstract:
Due to the remote location of many volcanoes, there is substantial uncertainty about the timing, amount and vertical distribution of volcanic ash released when they erupt. One approach to determine these properties is to combine prior estimates with satellite retrievals and simulations from atmospheric dispersion models to create posterior emission estimates, constrained by both the observations and the prior estimates, using a technique known as source inversion. However, the results are dependent not only on the accuracy of the prior assumptions, the atmospheric dispersion model and the observations used, but also on the accuracy of the meteorological data used in the dispersion simulations. In this study, we advance the source inversion approach by using an ensemble of meteorological data from the Met Office Global and Regional Ensemble Prediction System to represent the uncertainty in the meteorological data and apply it to the 2019 eruption of Raikoke. Retrievals from the Himawari-8 satellite are combined with NAME dispersion model simulations to create posterior emission estimates. The use of ensemble meteorology provides confidence in the posterior emission estimates and associated dispersion simulations that are used to produce ash forecasts. Prior mean estimates of fine volcanic ash emissions for the Raikoke eruption based on plume height observations are more than 15 times higher than any of the mean posterior ensemble estimates. In addition, the posterior estimates have a different vertical distribution, with 27 %–44 % of ash being emitted into the stratosphere compared to 8 % in the mean prior estimate. This has consequences for the long-range transport of ash, as deposition to the surface from this region of the atmosphere happens over long timescales. The posterior ensemble spread represents uncertainty in the inversion estimate of the ash emissions. For the first 48 h following the eruption, the prior ash column loadings lie outside an estimate of the error associated with a set of independent satellite retrievals, whereas the posterior ensemble column loadings do not. Applying a risk-based methodology to an ensemble of dispersion simulations using the posterior emissions shows that the area deemed to be of the highest risk to aviation, based on the fraction of ensemble members exceeding predefined ash concentration thresholds, is reduced by 49 %. This is compared to estimates using an ensemble of dispersion simulations using the prior emissions with ensemble meteorology. If source inversion had been used following the eruption of Raikoke, it would have had the potential to significantly reduce disruptions to aviation operations. The posterior inversion emission estimates are also sensitive to uncertainty in other eruption source parameters and internal dispersion model parameters. Extending the ensemble inversion methodology to account for uncertainty in these parameters would give a more complete picture of the emission uncertainty, further increasing confidence in these estimates.Quantifying the impact of meteorological uncertainty on emission estimates and the risk to aviation using source inversion for the Raikoke 2019 eruption
ATMOSPHERIC CHEMISTRY AND PHYSICS 22:13 (2022) 8529-8545
Abstract:
Due to the remote location of many volcanoes, there is substantial uncertainty about the timing, amount and vertical distribution of volcanic ash released when they erupt. One approach to determine these properties is to combine prior estimates with satellite retrievals and simulations from atmospheric dispersion models to create posterior emission estimates, constrained by both the observations and the prior estimates, using a technique known as source inversion. However, the results are dependent not only on the accuracy of the prior assumptions, the atmospheric dispersion model and the observations used, but also on the accuracy of the meteorological data used in the dispersion simulations. In this study, we advance the source inversion approach by using an ensemble of meteorological data from the Met Office Global and Regional Ensemble Prediction System to represent the uncertainty in the meteorological data and apply it to the 2019 eruption of Raikoke. Retrievals from the Himawari-8 satellite are combined with NAME dispersion model simulations to create posterior emission estimates. The use of ensemble meteorology provides confidence in the posterior emission estimates and associated dispersion simulations that are used to produce ash forecasts. Prior mean estimates of fine volcanic ash emissions for the Raikoke eruption based on plume height observations are more than 15 times higher than any of the mean posterior ensemble estimates. In addition, the posterior estimates have a different vertical distribution, with 27 %-44 % of ash being emitted into the stratosphere compared to 8 % in the mean prior estimate. This has consequences for the long-range transport of ash, as deposition to the surface from this region of the atmosphere happens over long timescales. The posterior ensemble spread represents uncertainty in the inversion estimate of the ash emissions. For the first 48 h following the eruption, the prior ash column loadings lie outside an estimate of the error associated with a set of independent satellite retrievals, whereas the posterior ensemble column loadings do not. Applying a risk-based methodology to an ensemble of dispersion simulations using the posterior emissions shows that the area deemed to be of the highest risk to aviation, based on the fraction of ensemble members exceeding predefined ash concentration thresholds, is reduced by 49 %. This is compared to estimates using an ensemble of dispersion simulations using the prior emissions with ensemble meteorology. If source inversion had been used following the eruption of Raikoke, it would have had the potential to significantly reduce disruptions to aviation operations. The posterior inversion emission estimates are also sensitive to uncertainty in other eruption source parameters and internal dispersion model parameters. Extending the ensemble inversion methodology to account for uncertainty in these parameters would give a more complete picture of the emission uncertainty, further increasing confidence in these estimates. Copyright:Volcanic SO2 layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
Atmospheric Chemistry and Physics Copernicus Publications 22:8 (2022) 5665-5683